Discrete Analyzers in the Environmental Laboratory

Introductioncontamination. For instance, the cadmium reduction
Think of your old manual Spectronic 20, or yournitrate test contains significant amounts of ammonia
direct reading spectrophotometer that you use inin the buffer reagent and phosphate in the color
your lab. You line up your samples in a row. In frontreagent. Using individual disposable cuvettes ensures
of them, you place some small sample cups orthat there is no contamination. Washing cuvettes, or
maybe even a series of cuvettes, and you pipette ausing a flow cell, means you can never be sure.
known amount of sample into each cup. You thenUsing disposable optical cuvettes is the only way you
add a reagent and somehow mix the reagent andcan guarantee no carryover between tests or
sample. You do this for each sample. You may havesamples. The concept is similar to use of disposable
more reagents to add so you repeat the wholepetri dishes, disposable pipette tips, and disposable
process until all reagents are added. Then you start ahypodermic needles. The discrete analyzer easily and
timer. When the timer beeps you know you have arapidly analyzes multiple tests on single sample
certain "time window" to read the absorbance (orsolutions. Only disposable individually contained
concentration) of your samples. You read by manuallyreactions ensure that there is no interaction between
transferring the color-developed sample to asamples or tests.
spectrometer cuvette, by using a peristaltic pump toLet the robot do your pipetting.
transfer the sample to a flow cell already in theWhen you manually pipette samples you, hopefully,
spectrometer, or by inserting the tube or cuvetteuse a different pipette per sample. If not, you will at
that you used to develop the sample color in. Then,least rinse it in between samples, and possibly with
you press a button to send the reading to a printer,sample prior to transferring your sample aliquot to
a computer program, or you manually record thethe sample container. This is to avoid carryover
reading onto a laboratory worksheet.between samples. A flow analyzer uses an auto
Did you shake and mix every sample exactly thesampler. The sampling probe immerses in the wash
same way every time? Will you mix them the samestation rinsing the outside of the probe, and pulls
way every day? Will every analyst run them exactlywash solution from the station and into the analytical
the same way you have?cartridge.
Is there color or turbidity in the samples? Should youA discrete analyzer also uses a probe; however, it
zero your instrument with each sample, or only withoperates differently than flow analyzers. A discrete
reagent water blanks?analyzer's level detect mechanism ensures that the
Is the exact time you read the final absorbanceprobe immerses into the sample or reagents no
critical?further than necessary to withdraw the required
The process described is what you are automatingsample aliquot. The probe then washes itself on the
by using a discrete analyzer. Instead of lining upoutside at the wash station and pushes the sample
samples, you are pouring aliquots into sample cupsor reagent out into the sample cuvette. Between
that are placed on an auto sampler tray. Instead ofdispenses, the probe pushes excess wash water out
transferring a known amount of sample to a cuvette,ensuring no carryover. In other words, unlike a flow
the discrete analyzer does. Instead of addingsystem that only pulls sample in one direction, the
reagents and mixing, the discrete analyzer does.sampling probe on a discrete analyzer is bidirectional
Instead of starting a timer, the discrete analyzerpulling reagent and sample into its internal tubing only
does. Instead of reading the absorbance, recordingfar enough to withdraw the correct volume and then
the reading, and calculating a result the discretedispensing it by pushing it out the other way.
analyzer does.The machine can think.
The analyzer has automated almost all the simpleWhen doing a manual test you know if you ran out
colorimetric methods for you. Sample volume isof reagent or sample. A flow analyzer does not
measured and dispensed exactly the same way,know. A flow analyzer could end up aspirating from
every time. Reagents are added and mixed exactlyempty sample cups or empty reagent bottles all night
the same way every time. The timer is set andlong and think it is still running samples. A discrete
absorbance is measured exactly the same wayanalyzer with level detection prevents this. The level
every time. Results are calculated exactly the samedetect mechanism is a capacitance detector that
way every time.senses the difference between liquid and air. The
The discrete analyzer pipettes, dilutes, adds reagents,discrete software calculates the volume of reagents
mixes, calibrates, measures, calculates, and reports alland samples based on the height of liquid. The
for you. You select a method by keyboard. There issoftware continuously monitors sample and reagent
no hardware to manually change, no cartridge tovolumes and will not continue the test when it
rinse out, no baselines to monitor, no wavelengthdetects that reagents or samples have "run out".
filters to change. Sample and reagent volumes areThe sampling depth on a flow analyzer is usually
determined by a selection in a computer program,adjustable by the user and is usually towards the
not by the internal diameter of a peristaltic pumpbottom of the sample vial. On a discrete analyzer,
tube.the depth the probe immerses in a sample solution is
The discrete analyzer has done a lot for you but ita result of programming or instrument design. The
cannot control nor do everything. It cannotdepth sampled on the OI Discrete analyzer is
accurately prepare the stock calibration standard fordetermined by the level detect mechanism and the
you, even though it can accurately dilute it. It cannotsample aliquot required for the test. For instance, if
guarantee the standards and samples were placed on200 micro liters is required the probe will immerse just
the auto sampler tray in the right order. It cannotbelow 200 micro liters as determined by the volume
prepare the reagents for you or guarantee theyof the cup and the liquid level detected and withdraw
were placed in the right order; however, it cana software-defined amount above 200 micro liters. In
monitor their purity and remind you where they areother words, the discrete analyzer samples from the
supposed to go. It cannot make sure you've enteredtop 300 micro liters of sample solution. The probe
the proper sample ID for each sample position,only immerses as far as it has to. This minimizes
however, it can guarantee that the result obtainedpotential carryover contamination, and speeds the
for that sample position is traceable to the ID youprocess. In this way dispensing and rinsing is fast and
entered. It cannot know the sample lot ID for eachthere is no sample or reagent carried to another on
standard or reagent, but if you enter those ID's intothe sides of the probe.
the software, it can guarantee traceability of thoseWhen sampling from the top of the sample cup
reagents with your sample sets.there is a risk of loss of a volatile analyte from the
The software and built in electronics constantlytop of the solution or the risk of the adsorption of
monitor and adjust lamp voltage so that absorbancean analyte from the laboratory air into the top of the
readings do not drift. Drift is common in flowsolution. For instance, trace cyanide in near neutral
analyzers because the peristaltic pump tubing deliverssolution can be slowly lost from the top layer of
reagents by proportion. The discrete analyzer deliverssample solution into the lab air. This is especially
the exact amount of sample and reagent every time.evident with lower concentrations such as 10 ppb.
These volumes do not change. The discrete analyzerGain of the analyte is possible as well. Ammonia is a
has a fixed path length if the discrete analyzer doescommon laboratory contaminant. Ammonia readily
not transfer color-developed sample to anotheradsorbs into acidified solutions. It is possible for
cuvette, or flow cell, for measurement. In addition, if,ammonia to be "pulled" from laboratory air into the
the discrete analyzer reads through the walls of thesample solution. A flow analyzer would not as readily
cuvette the calibration curve is usually more stabledetect this loss or gain because it samples from the
and or reproducible than your reagents andbottom of the sample cup.
standards.There are some drawbacks
Change your thoughts on calibrationA discrete analyzer reacts sample in a heated cup
Beer's law states that the absorbance is equal to thethat is open to allow the probe to dispense samples
absorbtivity times the path length times theand reagents. The heat increases reaction rates and
concentration. It seems, however, sometimes we dois especially important for chemistries such as
not believe that Beer's law is a law. I say thisammonia that are slow to develop color. In manual
because according to this law, the absorbtivity is atesting the reagents are added in open containers,
constant. When the path length is fixed (always thehowever, the container shape can vary and the
same), the path length is a constant as well makingcontainer can be capped during mixing, heating, and
the only variable the concentration. Therefore, youcolor reaction. When flow analyzers were first
prepare standards of a known concentration,introduced one of the key advantages that gained its
measure the absorbance and determine theacceptance over manual methods was that reactions
absorbtivity. Assuming you can prepare reagentsoccurred enclosed within the tubing limiting its
exactly the same way every time, measure theexposure to laboratory air. In this aspect, discrete
same volume every time, and incubate your samplesanalyzers are kind of a step backwards.
the same amount of time every time, there shouldThere are significant advantages.
be no reason to assume that the absorbtivity wouldSimilar to holding a color developing reaction in its
change. If the absorbtivity does not change, thenown container till it reaches a color maximum,
there is no reason to calibrate every day. Moreover,discrete analyzers can also hold intermediate reactions
if the absorbtivity is not changing, you could actuallyfor long periods of time without risk of carryover,
be introducing error every time you calibrate becausedilution into a carrier reagents, or excessive
you may not be taking into account random errorsdispersion. This can be especially useful in enzyme or
that occur between analysts or even with yourselfreduction reactions where reaction rates are slow. A
as you inadvertently vary your technique on aflow analyzer would require long delay coils resulting in
day-to-day basis.very complex SFA chemistry manifolds. Often
As mentioned previously, daily calibration is requiredelevated temperature is used to speed reactions, but
for continuous flow methods because flow methodsin some chemistry, there are limits to the maximum
proportion the reagents and sample using a peristaltictemperatures possible. Since discrete analyzer
pump. Those pump tubes are changing with timereactions are occurring in individually contained
changing the relative proportion of sample andcuvettes, the time delay between reagent additions
reagents. Flow analyzers are still incredibly accurate, iton discrete analyzers is limited only by software. This
is just you need to calibrate each time.is a significant advantage over flow chemistry.
Calibrating consumes time. Especially accurate onesIn manual methods, obviously, the operator prepares
where you took great care to ensure your standardsall the calibration standards from a stock solution,
and reagents are fresh.dilutes any QC samples from a stock solution, dilutes
A manual spectrometer does not necessarily requiresamples known to be over calibration prior to color
a calibration each time. Many methods written fordevelopment, and dilutes samples that were over
manual spectrometers merely say, "analyze a checkcalibration once he or she notices that they are.
standard with each sample set". In fact, the stabilityUnless you have an added auto-dilutor attached to
of the calibration curve is the underlying conceptyour flow analyzer, you will still be diluting standards
behind direct reading spectrophotometers and filterand over calibration samples. Auto-dilution is an
wheel methods. For many colorimetric tests, theintegral function of a discrete analyzer. The dilutions
stability of the curve far exceeds the stability of thecan be preset during sample table entry if you know
standards or the reagents. Some examples are nitritethat the samples need to be diluted. Methods can be
and phosphate.programmed such that they dilute every sample and
A discrete analyzer should not require dailystandard all the time, or the instrument can be
calibrations and should allow us to extrapolate moreprogrammed so that over calibration, samples are
the ion chromatography, gas chromatography, anddiluted and re analyzed.
manual direct reading spectrometer concept of theAn analyst changes a manual or flow method from
Continuing Calibration Verification, or CCV. Asone to the next by memory, or by referring to the
mentioned, the reason the discrete analyzer curvesSOP. How well this particular analyst performs the
are stable is that the robot exactly reproducesprocedure is dependent upon his mood, the time of
everything every time. You cannot do this becauseday, his experience with the method, the availability
you are not a robot, the discrete analyzer, however,of equipment, and many other unquantifiable
is.variables. It is possible to obtain good results and bad
A manual method uses more reagent and sampleresults by the same manually performed method. A
volume because we, as humans, cannot work easilyflow analyzer analyzes everything the same every
with small volumes. A flow system uses moretime assuming it is set up the same every time. This
reagent than a discrete analyzer because a flowassumption is valid with experienced flow analysis
instrument is continuously pumping reagent throughtechnicians; however, if the technician does not
the system.understand flow or if there are multiple users results
Discrete analyzers that measure the samplewill vary. Extensive training and documentation is
absorbance within the same container that thenecessary to guarantee that results conform to good
reaction occurred generate less waste thanautomated lab practices.
instruments that wash the vessel, or use a flow cell.The discrete analyzer method is selected by mouse
In fact, adequately rinsing a flow cell requiresclick when scheduling analyses on the sample tray.
significant rinsing between samples making the wasteThe method conditions do not change. In fact,
volume generated essentially equivalent to that of aassuming you have accurately calibrated your method
micro-flow Segmented Flow Analyzer, or Low Flowthe calibration is stored within the method. This
Flow Injection Analyzer.means that an untrained analyst that only knows
The discrete analyzer uses significantly less reagent,what buttons to press is able to obtain identical
and generates significantly less waste than manualresults to even the most experienced analyst.
methods. This chart illustrates an unscaled downMost analytes performed in an environmental
manual method using the exact volumes described incompliance laboratory cannot be bench spiked. If the
Standard Methods. The waste generated for theanalyte requires a preliminary distillation, digestion, or
manual method does not take into account washingextraction the spiking is done prior to the preliminary
of glassware. As mentioned earlier, an analyzer thatsample process. I realize that many labs do not distill
washes cuvettes or rinses a flow cell will generateammonia or Fluoride and I would argue that if you
more waste than indicated here.are reporting compliance testing for the clean water
Eliminate the possibility of contamination, or falseact you would better seriously consider changing your
positivesSOP. Other parameters that can't be spiked are
The discrete analyzer measuring the absorbance of athose that are too high to spike within the matrix
color reacted sample contained in individual cuvettes.without preliminary dilution, such as Ca, Mg, Cl, SO4,
Unlike flow analysis, there is no possibility ofand analytes like alkalinity that just are not spiked.
interaction between samples and unlike flow analysis;This shortens the list of potential analytes for the
the user can visually observe the reaction productautomatic spiking function to nitrite, phosphate,
during and after analysis.Sulfide, Chromium VI, and some others. On these, I
Using a discrete analyzer, the analyst can observedefer back to the previous slide and ask if the
the reaction during color development and after thepotential error is worth the risk for so few tests.
test is complete. The analyst can remove theSummary
reaction segments and verify that dispensed volumesBenefits of discrete analyzers include decreased
are repeatable, that there are no bubbles or turbidity,reagent consumption, decreased waste generated,
and that the color looks correct. A flow analyzerand ease of use among other things. The most
does not give the analyst the ability to visuallysignificant advantage of the discrete analyzer,
examine and qualitatively guarantee the accuracy ofhowever, is that it can eliminate the traditional
his or her results.concept of routine analysis and allow you to run
A discrete analyzer dispenses, reacts, incubates, andsamples as you receive them instead of storing them
measures all within the reaction cuvette withoutuntil there is enough sitting around to make a flow or
transferring to a flow cell. Analyzers that transfer toIC analysis worthwhile. If you take advantage of the
a flow cell are not "true" discrete analyzers, butcalibration stability of the discrete analyzer, and
instead, are hybrids between flow and discrete. Theaccurately prepare a calibration that can then be used
hybridization is done to achieve lower detection limits;by almost any analyst in subsequent uses an added
however, the advantage of the individually containedbenefit is that the results are the same regardless of
reaction and absence of carryover is lost. In addition,who uses the machine.
since these analyzers require as much rinse as a flowThink of those short holding time samples. The
analyzer to remove preceding samples, wastephosphate, the nitrites, the chromium VI, and residual
generation is as high as flow. Given this, and thechlorine. These analytes cause the environmental lab
increased possibility of environmental contamination orto stop everything just to get the analysis done on
analyte loss that occurs from open-air heatedtime. Think of the other analytes that come in
reactions, you may as well have a flow analyzer.periodically, but maybe not frequently. Possibly silica,
Chemical reactions occur in individually containedferrous iron and sulfide. How do you guarantee these
segmentstests followed the SOP? Instead of thinking of the
All discrete analyzers have reaction segments. Somediscrete analyzer as something to replace a flow
analyzers do chemical reactions in a cuvette segmentinstrument, think of it as something to supplement a
and then transfer the reacted sample to a flow cell.flow instrument. If you have hundreds of samples for
This type of analyzer is a hybrid of discrete and flow,one or two tests routinely and for the same analyte
and not a true discrete analyzer. A true discreteyou are not going to save money by switching these
analyzer reacts and measures the sample within thetests to a discrete analyzer. Where you will save
optical cuvette. Some analyzers wash the opticalmoney and great effort is removing unnecessary
cuvette between tests. Washing between testsstrain from the flow analyzer and your analysts by
enables more samples to be analyzed per cuvette;performing the non - routine or "rush" tests on a
however, the washing cannot guarantee that there isdiscrete analyzer. It is possible for the sample login
no residual contamination that remaining after theperson to analyze samples as received for almost
washing process. Other discrete analyzers utilizeevery colorimetric test that does not require a
disposable optical quality cuvettes.digestion. In other words, as soon as the sample is
Washing between tests enables more samples to belogged in it could be immediately run for nitrite,
analyzed per cuvette; however, the washing cannotphosphate, chromium VI, nitrate, ammonia, chloride,
guarantee that there is no residual contamination notand sulfate. In this example, instead of putting
completely removed by the washing process. Thissamples in a refrigerator to be gathered for analysis
residual contamination can come from precedingat a later time, they end up being run by ice chest
samples, or more likely, from the reagents used inand by client as soon as they are received.
processing the preceding samples. The built inIf everything is to run on the discrete analyzer, then
computerized checking of optical quality cannot verifycollect your samples in a vial that fits on the discrete
absence of chemical contamination.analyzer. You no longer need to transfer liquid from
Analyzers that use a flow cell still react samples incontainer A to auto sampler vial B, the sample bottle
some sort of cuvette. It is the number of reactioncan be the auto sampler vial. Not only does this save
vessels on the discrete analyzer that limit the numbertime, but it saves shipping as well. Instead of large ice
of tests that the discrete can run in a single walkchests, you use tiny mailers.
away operation. If the discrete analyzer has 100To summarize, the true advantage of a discrete
sample positions and 200 reaction cuvettes, then theanalyzer is that its built in features allow any analyst
analyzer can run 100 samples for 2 tests each. Theto get the same results every time. Discrete
discrete analyzer with the flow cell must rinse theanalyzers are very simple to use requiring minimal
flow cell between each sample, and rinse vigorouslysoftware training. Once set up for your laboratory,
between each test. Consider that a two-channel flowproperly applied methods allow you to modify your
analyzer can analyze 100 samples for two tests eachdaily routines and analyze samples as soon as they
in less than half the time as a discrete analyzer with acome in. Whether you are an environmental lab,
flow cell. Also, consider that the flow analyzerresearch, process control, or municipality discrete
generates no more waste than the discrete analyzeranalyzers can be used effectively in your operation.
with a flow cell. If the required testing is a lot ofCurrently, the full power of discrete analyzers is
samples for one or two tests it makes more senselimited by tradition and by regulation. Once we start
to use a flow analyzer.to develop methods for discrete analyzers instead of
Reagents can interfere as cross contaminationusing discrete analyzers to run methods developed
between samples. Using disposable individual reactionfor flow we will be able to see greater throughput,
cuvettes completely eliminates the possibility ofless variability, and lower MDL.